Phys. Status Solidi B (2014)
Time-resolved magneto-optics is a well-established optical pump–probe technique to generate and to probe spin coherence in semiconductors. By this method, spin dephasing times T₂* can easily be determined if their values are comparable to the available pump–probe delays. If T₂* exceeds the laser repetition time, however, resonant spin amplification (RSA) can equally be used to extract T₂* image. We demonstrate that in ZnO these techniques have several tripping hazards resulting in deceptive values for T₂* and show how to avoid them. We show that the temperature dependence of the amplitude ratio of two separate spin species can easily be misinterpreted as a strongly temperature-dependent T₂* of a single spin ensemble, while the two spin species have T₂* values, which are nearly independent of temperature. Additionally, consecutive pump pulses can significantly diminish the spin polarization, which remains from previous pump pulses. While this barely affects T₂* values extracted from delay line scans, it results in seemingly shorter inline image values in RSA.